Bio-inspired model of photosystem II: supramolecular assembly of an electron mediator into an SnO2 photoanode co-sensitized by a porphyrin photosensitizer and ruthenium molecular catalyst

文献情報

出版日 2018-01-02

DOI 10.1039/C7SE00515F

インパクトファクター 6.367

著者

Yong Na, Siwen Miao, Li Zhou, Peicheng Wei, Yang Cao

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要旨

A bio-inspired electron transfer mediator was incorporated via a Zr4+ ion linkage into a photoanode assembled from a porphyrin photosensitizer displaying broad spectral coverage in the visible region and a ruthenium water oxidation catalyst. Incorporation of the electron mediator suppressed unwanted charge recombination and facilitated the transfer of charge from aqueous electrolyte to the photoanode, resulting in an increase in the photocurrent. A remarkable enhancement of faradaic efficiency for oxygen evolution upon introduction of the mediator was observed in the photoelectrochemical cell.

掲載誌

Sustainable Energy & Fuels

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Bio-inspired model of photosystem II: supramolecular assembly of an electron mediator into an SnO2 photoanode co-sensitized by a porphyrin photosensitizer and ruthenium molecular catalyst

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