Fe(0) powder-catalyzed one-pot reaction: concurrent living radical polymerization and click chemistry for topological polymers

文献情報

出版日 2015-05-26

DOI 10.1039/C5PY00654F

インパクトファクター 5.582

著者

Hui Zhu, Zhenbiao Zhang, Nianchen Zhou, Xiulin Zhu

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要旨

Fe(0) powder-catalyzed one-pot reaction was successfully employed to design linear and star polymers in a well-controlled manner by combining ambient temperature living radical polymerization and click chemistry. The polymerization behavior possessed the characteristics of “living”/controlled radical polymerization: the first-order kinetic plots, narrow molecular weight distribution (PDI < 1.4), the linear relationship between molecular weights and the monomer conversions and the successful chain-extension with a NIPAAM monomer. Furthermore, the NMR and MALDI-TOF-MS data indicated that the Fe(0)-catalyzed one-pot strategy is different from our reported Cu(0)-catalyzed one-pot strategies to make the targeted polymers.

掲載誌

Polymer Chemistry

CiteScore: 8.6

自己引用率: 7.3%

年間論文数: 457

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Fe(0) powder-catalyzed one-pot reaction: concurrent living radical polymerization and click chemistry for topological polymers

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