A PEDOT:PSS nanocomposite film doped with black phosphorus modified with silver nanoparticles for wearable photothermoelectric generators

文献情報

出版日 2023-10-26

DOI 10.1039/D3TA05836K

インパクトファクター 12.732

著者

Chia-Hao Tsai, Shih-Hung Tung, Jhih-Min Lin

原文を見る

要旨

Photothermoelectric (PTE) materials have gained significant attention as a promising avenue for converting light into electricity. Herein, the PTE properties of poly(3,4-ethylenedioxythiophene):poly(styrenesulfonate) (PEDOT:PSS) are enhanced by introducing black phosphorus nanosheets (BP NSs) modified with silver nanoparticles (Ag@BP). Under 100 mW cm−2 illumination, the resulting PEDOT:PSS/Ag@BP nanocomposite film (P_Ag@BP) exhibits an output voltage of 528.4 μV compared to 300.9 μV for the PEDOT:PSS film. This is attributed to (i) the enhanced photothermal performance of P_Ag@BP, which generates a temperature difference of 18 °C under 100 mW cm−2 illumination compared to 10 °C for the PEDOT:PSS film and (ii) the enhanced thermoelectric performance of P_Ag@BP, with an increased power factor of 107.2 μW m−1 K−2 compared to 32.9 μW m−1 K−2 for the PEDOT:PSS film. Moreover, a photothermoelectric generator (PTEG) consisting of 36 legs of P_Ag@BP exhibits an open circuit voltage of 16.1 mV, a short circuit current of 47.9 μA, and an output power of 192.6 nW under 120 mW cm−2 illumination. Furthermore, when the PTEG is worn on the forearm and exposed to sunlight, it generates an output voltage of 9.2 mV, thus showcasing its potential application in wearable energy harvesting devices.

掲載誌

Journal of Materials Chemistry A

CiteScore: 19.5

自己引用率: 4.7%

年間論文数: 2211

Journal of Materials Chemistry A, B & C cover high quality studies across all fields of materials chemistry. The journals focus on those theoretical or experimental studies that report new understanding, applications, properties and synthesis of materials. The journals have a strong history of publishing quality reports of interest to interdisciplinary communities and providing an efficient and rigorous service through peer review and publication. The journals are led by an international team of Editors-in-Chief and Associate Editors who are all active researchers in their fields. Journal of Materials Chemistry A, B & C are separated by the intended application of the material studied. Broadly, applications in energy and sustainability are of interest to Journal of Materials Chemistry A, applications in biology and medicine are of interest to Journal of Materials Chemistry B, and applications in optical, magnetic and electronic devices are of interest to Journal of Materials Chemistry C. More than one Journal of Materials Chemistry journal may be suitable for certain fields and researchers are encouraged to submit their paper to the journal that they feel best fits for their particular article. Example topic areas within the scope of Journal of Materials Chemistry A are listed below. This list is neither exhaustive nor exclusive. Artificial photosynthesis Batteries Carbon dioxide conversion Catalysis Fuel cells Gas capture/separation/storage Green/sustainable materials Hydrogen generation Hydrogen storage Photocatalysis Photovoltaics Self-cleaning materials Self-healing materials Sensors Supercapacitors Thermoelectrics Water splitting Water treatment

A PEDOT:PSS nanocomposite film doped with black phosphorus modified with silver nanoparticles for wearable photothermoelectric generators

文献情報

おすすめジャーナル

関連文献

Photovoltage improvements and recombination suppression by montmorillonite addition to PEO gel electrolyte for dye-sensitized solar cells

Mesoscopic non-equilibrium thermodynamics of non-isothermal reaction-diffusion

Interactions of TRIS [tris(hydroxymethyl)aminomethane] and related buffers with peptide backbone: Thermodynamic characterization

Structure–activity relationship (SAR) for the prediction of gas-phase ozonolysis rate coefficients: an extension towards heteroatomic unsaturated species

Rules for selectivity in oxidation processes on RuO2(110)

Should negative electron affinities be used for evaluating the chemical hardness?

Reentrant behavior of grafted poly(sodium styrenesulfonate) chains investigated with a quartz crystal microbalance

Synthesis and enhanced photocatalytic performance of graphene-Bi2WO6 composite

In situ surface-enhanced Raman scattering and X-ray photoelectron spectroscopic investigation of coenzyme Q10 on silver electrode

Synthesis and photophysics of monodisperse co-oligomers consisting of alternating thiophene and perylene bisimide‡

こちらもおすすめ

2,3-スチオエポキシマドルを取り扱う際の実験室安全事項は何ですか？

6-氟-2-氨基苯酚の主な用途は何ですか？

BOC-S-3-アミニ-4-(4-メチオキシベンチル)-ブタン酸の代替品はありますか？

Methyl 2-(chloromethyl)-3-nitrobenzoate（1218910-61-2）の代替品はありますか？

（2R)-2-アミノ-N-ベンジル-3-ヒドロキシプロパナミドを含む廃棄物はどのように処理すべきですか？

6,7-二氢-咪唑並[1,2-a]ピリドイン-8(5h)-酮はどのように合成されますか？

エチル(3R)-3-ピロリジニル酢酸水和塩とは何ですか？

（2S）-{[(2-メチルエチルオキシ]カルボニル}アミノ)[2-(トリアフルオロメチルフェニル]エチカシック酸の物理化学的性質は何ですか？

2-ブロモ-1-(2-メチル-2-プロパニル)-4-ニトロベンゼンはどのように保存すればよいですか？

1-[(4-硝基フェニル)スルホニル]-1H-1,2,4-三唑の市場動向や研究トレンドはどうですか？

掲載誌

Journal of Materials Chemistry A

おすすめ化合物

2-Cyano-2-methylpropanamide

4-(Bromomethyl)-1-cyclohexyl-2-(trifluoromethyl)benzene

6,6-Dimethylbicyclo[3.1.1]hept-2-ene-2-carbaldehyde

(9S,10E,12Z)-9-Hydroxy-10,12-octadecadienoic acid

Ethyl 2,4-bis(trifluoromethyl)-5-pyrimidinecarboxylate

おすすめサプライヤー