Engineering surface lattice hydroxyl groups toward highly efficient photocatalytic methane coupling

文献情報

出版日 2023-12-22

DOI 10.1039/D3CC04645A

インパクトファクター 6.222

著者

Zili Ma, Yihong Chen, Chao Gao

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要旨

Nb3O7(OH) containing abundant surface lattice hydroxyl groups, combining with loaded Au nanoparticles as the cocatalyst, was employed as a photocatalyst enabling highly efficient photocatalytic CH4 coupling to C2H6 under mild conditions. In situ spectroscopy technique revealed that the surface lattice hydroxyl groups play a vital role in promoting the activation of CH4 to produce the methoxy intermediates, contributing to significantly enhanced catalytic performance for CH4 conversion.

掲載誌

Chemical Communications

CiteScore: 8.6

自己引用率: 4.7%

年間論文数: 2458

ChemComm publishes urgent research which is of outstanding significance and interest to experts in the field, while also appealing to the journal’s broad chemistry readership. Our communication format is ideally suited to short, urgent studies that are of such importance that they require accelerated publication. Our scope covers all topics in chemistry, and research at the interface of chemistry and other disciplines (such as materials science, nanoscience, physics, engineering and biology) where there is a significant novelty in the chemistry aspects. Major topic areas covered include: Analytical Chemistry Catalysis Chemical Biology and medicinal chemistry Computational Chemistry and Machine Learning Energy and sustainable chemistry Environmental Chemistry Green Chemistry Inorganic Chemistry Materials Chemistry Nanoscience Organic Chemistry Physical Chemistry Polymer Chemistry Supramolecular Chemistry

Engineering surface lattice hydroxyl groups toward highly efficient photocatalytic methane coupling

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