Toward a tunable synthetic [FeFe] hydrogenase mimic: single-chain nanoparticles functionalized with a single diiron cluster

文献情報

出版日 2015-09-10

DOI 10.1039/C5PY01196E

インパクトファクター 5.582

著者

C. A. Tooley, S. Pazicni

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要旨

We report two novel “clickable” [(μ-S2C2H4NR)Fe2(CO)6] complexes and their incorporation into single-chain nanoparticles. Variations in the characteristic iron–carbonyl stretching bands caused by the polymer scaffolds confirmed changes in the symmetry and electronics of the complexes. This represents the first SCNP-based model of a metalloenzyme bearing a single, bioinspired active site.

掲載誌

Polymer Chemistry

CiteScore: 8.6

自己引用率: 7.3%

年間論文数: 457

Polymer Chemistry welcomes submissions in all areas of polymer science that have a strong focus on macromolecular chemistry. Manuscripts may cover a broad range of fields, yet no direct application focus is required.

Toward a tunable synthetic [FeFe] hydrogenase mimic: single-chain nanoparticles functionalized with a single diiron cluster

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Development of thermosensitive copolymers of poly(2-methoxyethyl acrylate-co-poly(ethylene glycol) methyl ether acrylate) and their nanogels synthesized by RAFT dispersion polymerization in water

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