Terminal functional glycopolymersvia a combination of catalytic chain transfer polymerisation (CCTP) followed by three consecutive click reactions

文献情報

出版日 2012-02-03

DOI 10.1039/C2PY20013A

インパクトファクター 5.582

著者

Qiang Zhang, Stacy Slavin, Mathew W. Jones, Alice J. Haddleton, David M. Haddleton

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要旨

The combination of catalytic chain transfer polymerisation (CCTP) with both thiol-ene and copper catalysed alkyne azide coupling (CuAAC) click chemistry has been employed to give a new route to functional glycopolymers for applications in bioconjugation and biological targeting. Ring opening of poly(glycidyl methacrylate) with sodium azide and subsequent reaction with alkyne functional carbohydrates, as prepared by Fischer glycosylation, has been exploited. This combination of a range of efficient chemistry gives a route to multi gram quantities of glycopolymers avoiding the need for living radical polymerisation chemistry.

掲載誌

Polymer Chemistry

CiteScore: 8.6

自己引用率: 7.3%

年間論文数: 457

Polymer Chemistry welcomes submissions in all areas of polymer science that have a strong focus on macromolecular chemistry. Manuscripts may cover a broad range of fields, yet no direct application focus is required.

Terminal functional glycopolymersvia a combination of catalytic chain transfer polymerisation (CCTP) followed by three consecutive click reactions

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